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The quantum twisting microscope: A new lens on quantum materials

A clever take on the science of twistronics offers new ways of exploring quantum phenomena

One of the striking aspects of the quantum world is that a particle, say, an electron, is also a wave, meaning that it exists in many places at the same time. In a new study, reported today in Nature, researchers from the Weizmann Institute of Science make use of this property to develop a new type of tool – the quantum twisting microscope (QTM) – that can create novel quantum materials while simultaneously gazing into the most fundamental quantum nature of their electrons. The study’s findings may be used to create electronic materials with unprecedented functionalities.

The QTM involves the “twisting,” or rotating, of two atomically-thin layers of material with respect to one another. In recent years, such twisting has become a major source of discoveries. It began with the discovery that placing two layers of graphene, one-atom-thick crystalline sheets of carbon, one atop the other with a slight relative twist angle, leads to a “sandwich” with unexpected new properties. The twist angle turned out to be the most critical parameter for controlling the behavior of electrons: Changing it by merely one-tenth of a degree could transform the material from an exotic superconductor into an unconventional insulator. But critical as it is, this parameter is also the hardest to control in experiments. By and large, twisting two layers to a new angle requires building a new “sandwich” from scratch, a process that is very long and tedious.

“Our original motivation was to solve this problem by building a machine that could continuously twist any two materials with respect to one another, readily producing an infinite range of novel materials,” says team leader Prof. Shahal Ilani of Weizmann’s Condensed Matter Physics Department. “However, while building this machine, we discovered that it can also be turned into a very powerful microscope, capable of seeing quantum electronic waves in ways that were unimaginable before.”

An animation showing the quantum twisting microscope in action. Electrons tunnel from the probe (inverted pyramid at the top) to the sample (bottom) as quantum mechanical waves (red)

Creating a quantum picture

Pictures have long played a central role in scientific discovery. Light microscopes and telescopes routinely provide images that allow scientists to gain a deeper understanding of biological and astrophysical systems. Taking pictures of electrons inside materials, on the other hand, has for many years been notoriously hard, owing to the small dimensions involved. This was transformed some 40 years ago with the invention of the scanning tunneling microscope, which earned its developers the 1986 Nobel Prize in Physics. This microscope uses an atomically sharp needle to scan the surface of a material, measuring the electric current and gradually building an image of the distribution of electrons in the sample.

“Many different scanning probes have been developed since this invention, each measuring a different electronic property, but all of them measure these properties at one location at a time. So, they mostly see electrons as particles, and can only indirectly learn about their wave nature,” explains Prof. Ady Stern from the Weizmann Institute, who took part in the study along with three other theoretical physicists from the same department: Profs. Binghai Yan, Yuval Oreg and Erez Berg. “As it turned out, the tool that we have built can visualize the quantum electronic waves directly, giving us a way to unravel the quantum dances they perform inside the material,” Stern says.

Twisting (l-r, clockwise): Jiewen Xiao, Prof. Ady Stern, Prof. Shahal Ilani, Prof. Erez Berg, Prof. Binghai Yan, Dr. John Birkbeck and Alon Inbar. On the wall: Schroedinger's equation for the electron's wave function

Spotting an electron in several places at once

“The trick for seeing quantum waves is to spot the same electron in different locations at the same time,” says Alon Inbar, a lead author on the paper. “The measurement is conceptually similar to the famous two-slit experiment, which was used a century ago to prove for the first time that electrons in quantum mechanics have a wave nature,” adds Dr. John Birkbeck, another lead author. “The only difference is that we perform such an experiment at the tip of our scanning microscope.”

To achieve this, the researchers replaced the atomically sharp tip of the scanning tunneling microscope with a tip that contains a flat layer of a quantum material, such as a single layer of graphene. When this layer is brought into contact with the surface of the sample of interest, it forms a two-dimensional interface across which electrons can tunnel at many different locations. Quantum mechanically, they tunnel in all locations simultaneously, and the tunneling events at different locations interfere with each other. This interference allows an electron to tunnel only if its wave functions on both sides of the interface match exactly. “To see a quantum electron, we have to be gentle,” says Ilani. “If we don’t ask it the rude question ‘Where are you?’ but instead provide it with multiple routes to cross into our detector without us knowing where it actually crossed, we allow it to preserve its fragile wave-like nature.”

Close-up diagram of the quantum twisting microscope in action. Electrons tunnel from the probe (inverted pyramid at the top) to the sample (bottom) in several places at once (green vertical lines), in a quantum coherent manner

Twist and tunnel

Generally, the electronic waves in the tip and the sample propagate in different directions and therefore do not match. The QTM uses its twisting capability to find the angle at which matching occurs: By continuously twisting the tip with respect to the sample, the tool causes their corresponding wave functions to also twist with respect to one another. Once these wave functions match on both sides of the interface, tunneling can occur. The twisting therefore allows the QTM to map how the electronic wave function depends on momentum, similarly to the way lateral translations of the tip enable the mapping of its dependence on position. Merely knowing at which angles electrons cross the interface supplies the researchers with a great deal of information about the probed material. In this manner they can learn about the collective organization of electrons within the sample, their speed, energy distribution, patterns of interference and even the interactions of different waves with one another.

Prof. Yuval Oreg

A new twist on quantum materials

“Our microscope will give scientists a new kind of ‘lens’ for observing and measuring the properties of quantum materials,” says Jiewen Xiao, another lead author.

The Weizmann team has already applied their microscope to studying the properties of several key quantum materials at room temperature and is now gearing up toward doing new experiments at temperatures of a few kelvins, where some of the most exciting quantum mechanical effects are known to take place.

Peering so deeply into the quantum world can help reveal fundamental truths about nature. In the future, it might also have a tremendous effect on emerging technologies. The QTM will provide researchers with access to an unprecedented spectrum of new quantum interfaces, as well as new “eyes” for discovering quantum phenomena within them.

 

Prof. Shahal Ilani’s research is supported by the Helen and Martin Kimmel Award for Innovative Investigation; the Sagol Weizmann-MIT Bridge Program; and the Rosa and Emilio Segre Research Award.

Prof. Ady Stern is head of the Schwartz Reisman Institute for Theoretical Physics.

Prof. Yuval Oreg is head of the Maurice and Gabriella Goldschleger Center for Nanophysics and the incumbent of the Lady Davis Professorial Chair of Physics.

 

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